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Issue
Korean Journal of Chemical Engineering,
Vol.38, No.10, 2034-2046, 2021
Photocatalytic removal of Rhodamine B in water using g-C3N4/MIL-53(Fe) material under LED visible light with persulfate activation
Dung NT, Hiep NV, Nguyen MB, Thao VD, Huy NN
Photocatalysis is usually considered as one of the most effective methods for treating non-biodegradable pollutants commonly found in textile wastewater. In this study, the photocatalyst of g-C3N4/MIL-53(Fe) was synthesized by the hydrothermal method and applied for the removal of Rhodamine B (RhB) in water. The photocatalytic material was characterized by X-ray diffraction, Fourier-transform infrared spectroscopy, scanning electron microscopy, energy-dispersive X-ray spectroscopy, Brunauer-Emmett-Teller analysis, UV-Vis diffuse reflectance spectroscopy, and X-ray photoelectron spectroscopy. The results showed that the g-C3N4 doped MIL-53(Fe) with 97 wt% of MIL-53(Fe) works effectively under visible light and the presence of oxidants (Na2S2O8). RhB removal efficiency can be more than 99% with 20mg/L of RhB, 300mg/L of catalyst, 200mg/L of Na2S2O8, and pH 3. In addition, the photocatalytic degradation mechanism of RhB with g-C3N4/MIL-53(Fe) was also proposed, which could be improved and studied for a wide range of applications in textile wastewater treatment.
Keywords: Rhodamine B; g-C3N4; MIL-53(Fe); Photocatalysis; Visible Light
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