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Issue
Korean Journal of Chemical Engineering,
Vol.38, No.2, 442-453, 2021
Nature-mimicking fabrication of antifouling photocatalytic membrane based on Ti/BiOI and polydopamine for synergistically enhanced photocatalytic degradation of tetracycline
Cui Y, Yang L, Yan Y, Wang Z, Zheng J, Li B, Feng Y, Li C, Meng M
The photocatalytic efficiency of conventional blending photocatalytic membranes suffers a significant reduction due to effective photocatalyst embedded in membrane matrix. Therefore, in this study, inspired by the bioadhesive technology of polydopamine (pDA), a novel Ti doped bismuth oxyiodide (BiOI)-polydopamine (pDA)-coated cellulose acetate (CA) (Ti/BiOI-pDA/CA) photocatalytic nanocomposite membranes were successfully developed for effective removal of tetracycline (TC). The Ti/BiOI-pDA/CA nanocomposite membranes displayed very high photocatalytic activity toward TC (about 98% after 120 min) under visible light irradiation and superior photodegradation kinetics (k=0.03214 min-1). The removal rate of Ti/BiOI/-pDA/CA nanocomposite membranes under dynamic cyclic degradation system could be further improved, giving TC removal efficiency of 91% in 60min. Remarkably, the permeate flux, flux recovery ratio (FRR), reversible fouling (Rr), irreversible fouling (Rir) and the total fouling ratio (Rt) revealed the Ti/BiOI-pDA/CA nanocomposite membranes had excellent antifouling performance. In addition, the Ti/ BiOI-pDA/CA nanocomposite membranes exhibited excellent stability and reusability. Therefore, this work gives insight into the effective removal of TC wastewater and has a great potential for new generation of high-performance photocatalytic membranes for practical wastewater treatment in the future.
Keywords: Flower-like Ti/BiOI; pDA/CA Hybrid Membrane; Fouling Mechanismm Photodegradation
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[Cited By]
  1. Khane A, Tahmasebi N, Kaboli HS, Korean Journal of Chemical Engineering, 39(5), 1248, 2022
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