Korean Journal of Chemical Engineering, Vol.38, No.1, 187-194, 2021
Morphological improvement of CH3NH3PbI3 films using blended solvents for perovskite solar cells
Perovskite solar cells with the structure of glass/florine-doped tin oxide (FTO)/electron transfer layer (ETL)/ perovskite/hole transfer layer (HTL)/Ag were fabricated. The effects of blending solvents and thermal annealing on the surface morphology, structural, and optical properties of perovskite (CH3NH3PbI3) active layer were investigated. The active layer was optimized by adding 2-butanol (2-BTA) as an eco-friendly solvent into methyl ammonium iodide (MAI) solution used for spin coating on PbI2/(dimethylformamide (DMF)+dimethyl sulfoxide (DMSO)) film in the second step. The resulting morphology of CH3NH3PbI3 films was smooth and pinholes in the films were also reduced without change in the structure. The effects of thermal annealing on the surface morphology and structural properties of active layer were also studied. The fabricated device for the optimized condition showed the maximum power conversion efficiency (PCE) of ~8.6%.
[References]
Jacobsson TJ, Correa-Baena JP, Pazoki M, Saliba M, Schenk K, Gratzel K, Hagfeldt A, Energy Environ. Sci. , 9 , 1706, 2016
Park NG, Gratzel M, Miyasaka T, Zhu K, Emery K, Nat. Energy , 1 , 16152, 2016
Deng WQ, Yuan ZT, Liu SH, Yang ZL, Li J, Wang EJ, Wang XB, Li JH, J. Power Sources , 432 , 112, 2019
Galkowski K, Mitioglu A, Miyata A, Plochocka P, Portugall O, et al., Energy Environ. Sci. , 9 , 962, 2016
Anuratha KS, Peng HS, Xiao YM, Su TS, Wei TC, Lin JY, Electrochim. Acta , 295 , 662, 2019
Ogomi Y, Morita A, Tsukamoto S, Saitho T, Fujikawa N, et al., J. Phys. Chem. Lett. , 5 , 1004, 2014
Im JH, Kim HS, Park NG, APL Mater. , 2 , 081510, 2014
Im JH, Lee CR, Lee JW, Park SW, Park NG, Nanoscale , 3 , 4088, 2011
Kojima A, Teshima K, Shirai Y, Miyasaka T, J. Am. Chem. Soc. , 131 (17), 6050, 2009
Hou Y, Aydin E, De Bastiani M, Xiao CX, Isikgor FH, Xue DJ, Chen B, Chen H, Bahrami B, Chowdhury AH, Johnston A, Baek SW, Huang ZR, Wei MY, Dong YT, Troughton J, Jalmood R, Mirabelli AJ, Allen TG, Van Kerschaver E, Saidaminov MI, Baran D, Qiao QQ, Zhu K, , Science , 367 (6482), 1135, 2020
Sun X, Zhang C, Chang J, Yang H, Xi H, Lu G, Chen D, Lin Z, Lu X, Zhang J, Hao Y, Nano Energy , 28 , 417, 2016
Lee MM, Teuscher J, Miyasaka T, Murakami TN, Snaith HJ, Science , 338 (6107), 643, 2012
Arivazhagan V, Xie JS, Yang ZR, Hang PJ, Parvathi MM, Xiao K, Cui C, Yang DR, Yu XG, Sol. Energy , 181 , 339, 2019
Chen Q, Zhou HP, Hong ZR, Luo S, Duan HS, Wang HH, Liu YS, Li G, Yang Y, J. Am. Chem. Soc. , 136 (2), 622, 2014
Duong TT, Hoang PH, Nhan LT, Van Duon L, Nam MH, Tuan L, Curr. Appl. Phys. , 19 (11), 1266, 2019
Peng X, Yuan J, Shen S, Gao M, Chesman ASR, Yin H, Cheng J, Zhang Q, Angmo D, Adv. Funct. Mater. , 27 , 170370, 2017
Wang M, Feng Y, Bian J, Liu H, Shi Y, Chem. Phys. Lett. , 692 , 2017
Gardner KL, Tait JG, Merckx T, Qiu W, Paetzold UW, Kootstra L, et al., Adv. Eng. Mater. , 6 , 160038, 2016
Jeon NJ, Noh JH, Kim YC, Yang WS, Ryu S, Il Seol S, Nat. Mater. , 13 (9), 897, 2014
Guillen E, Ramos FJ, Anta JA, Ahmad S, J. Phys. Chem. C , 118 , 22913, 2014
Im JH, Jang IH, Pellet N, Gratzel M, Park NG, Nat. Nanotechnol. , 9 (11), 927, 2014
Liu DY, Yang JL, Kelly TL, J. Am. Chem. Soc. , 136 (49), 17116, 2014
Zhang H, Mao J, He H, Zhang D, Zhu L, Xie F, Wong K, Gratzel M, Choy W, Adv. Eng. Mater. , 5 , 150135, 2015
Park BW, Kedem N, Kulbak M, Lee D, Yang W, Jeon N, Seo J, et al., Nat. Commun. , 9 , 3301, 2018
Gujar TP, Unger T, Schonleber A, Fried M, Panzer F, van Smaalen S, Kohler A, Thelakkat M, Phys. Chem. Chem. Phys. , 20 , 605, 2018
Li G, Zhang T, Zhao Y, J. Mater. Chem. A , 3 , 19674, 2015
Shi Y, Wang X, Zhang H, Li B, Lu H, Ma T, Hao C, J. Mater. Chem. A , 3 , 22191, 2015
Chiang CH, Nazeeruddin M, Gratzel M, Wu CG, Energy Environ. Sci. , 10 , 808, 2017
Su LJ, Xiao YM, Han GY, Lu LP, Li HG, Zhu ML, J. Power Sources , 426 , 11, 2019
Abzieher T, Mathies F, Hetterich M, Welle A, Gerthsen D, Lemmer U, Paetzold UW, Powalla M, Phys. Status Solidi A-Appl. Res. , 214 , 170050, 2017
Kosmatos KO, Theofylaktos L, Giannakaki E, Deligiannis D, Konstantakou M, Stergiopoulos T, Energy Environ. Mater. , 2 , 79, 2019
Tseng ZL, Chiang CH, Wu CG, Sci. Rep. , 5 , 13211, 2015
Barbe J, Newman M, Lilliu S, Kumar V, Lee HKH, Charbonneau C, Rodenburg C, Lidzey D, Tsoi WC, J. Mater. Chem. A , 6 , 23010, 2018
Yang S, Zheng YC, Hou Y, Chen X, Chen Y, Wang Y, Zhao H, Yang HG, Chem. Mater. , 26 , 6705, 2014
Fu YP, Meng F, Rowley MB, Thompson BJ, Shearer MJ, Ma DW, Hamers RJ, Wright JC, Jin S, J. Am. Chem. Soc. , 137 (17), 5810, 2015
Le TTT, Le N, Pallavolu MR, Jeon YC, Jeong DS, Pejjai B, Reddy VRM, Truong NTN, Park CH, Korean J. Chem. Eng. , 36 (12), 2110, 2019
Chen LC, Chen JC, Cheng-Chiang C, Wu CG, Nanoscale Res. Lett. , 10 , 1020, 2015
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