Korean Journal of Chemical Engineering, Vol.38, No.1, 135-143, 2021
Facile synthesis of polyethyleneimine@Fe3O4 loaded with zirconium for enhanced phosphate adsorption: Performance and adsorption mechanism
Coating superparamagnetic iron oxide particles, i.e., Fe3O4, as adsorbents have major advantages over bare adsorbents for water treatment. As a versatile material, zirconium has been extensively studied for phosphate removal. In this study, the Fe3O4 core was pre-coated with branched polyethyleneimine (PEI) first, and then loaded with zirconium to result in a highly selective adsorbent (i.e., Zr-PEI@Fe3O4) for phosphate with a greatly broadened pH range. Scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS), BET surface area, and magnetization were used to characterize the resulting adsorbent and to explore the underlying adsorption mechanism. The adsorption performance of Zr-PEI@Fe3O4 toward phosphate was performed by batch experiment. The results showed that Freundlich model better fit the adsorption isotherms, while the Elovich equation better described the kinetic process. The maximum adsorption capacity of dephosphorization 32.2mgㆍg-1 (according to P element) emerged in the condition of 1.0 gㆍL-1 and pH at 2 with 303 K. The process was spontaneous and endothermic. Zr PEI@Fe3O4 has the potential to remove phosphate from solution due to its easy separation and some good adsorption property.
[References]
Mayer BK, Gerrity D, Rittmann BE, Reisinger D, Brandt-Williams S, Crit. Rev. Environ. Sci. Technol. , 43 , 409, 2013
Axinte O, Badescu IS, Stroe C, Neacsu V, Neacsu L, Bulgariu D, Environ. Eng. Manage. J. , 14 , 559, 2015
Yang Y, Shi X, Ballent W, Mayer BK, Water Environ. Res. , 89 , 2122, 2017
Peng LH, Dai H, Wu Y, Peng Y, Lu X, Chemosphere , 197 , 768, 2018
Xu X, Gao BY, Jin B, Yue QY, J. Mol. Liq. , 215 , 565, 2016
Wu BL, Wan J, Zhang YY, Pan BC, Lo IMC, Environ. Sci. Technol. , 54 , 50, 2020
Kumar PS, Korving L, van Loosdrecht MCM, Witkamp GJ, Water Res. X , 4 , 100029, 2019
Bhatnagar A, Kumar E, Sillanpaa M, Chem. Eng. J. , 171 (3), 811, 2011
Wang Z, Xing MC, Fang WK, Wu DY, Appl. Surf. Sci. , 366 , 67, 2016
Sarkar A, Biswas SK, Pramanik P, J. Mater. Chem. , 20 , 4417, 2010
Wang WJ, Zhou J, Wei D, Wan HQ, Zheng SR, Xu ZY, Zhu DQ, J. Colloid Interface Sci. , 407 , 442, 2013
Pham ALT, Sedlak DL, Doyle FM, Appl. Catal. B: Environ. , 126 , 258, 2012
Wang W, Zhang H, Zhang L, Wan H, Zheng S, Xu Z, Colloids Surf. A: Physicochem. Eng. Asp. , 469 , 100, 2015
An FQ, Gao BJ, J. Hazard. Mater. , 145 (3), 495, 2007
Huang BY, Liu YG, Li B, Wang H, Zeng G, RSC Adv. , 9 , 32462, 2019
Fu CC, Tran HN, Chen XH, Juang RS, J. Ind. Eng. Chem. , 11 , 33, 2019
Han RP, Fang LY, Li XY, Han MY, Zhang Z, J. Zhengzhou U. , 40 (2), 59, 2019
Gu YF, Liu MY, Yang MM, Wang WL, Zhang SS, Han RP, Desalin. Water Treat. , 138 , 368, 2019
Noreen S, Bhatti HN, Iqbal M, Hussain F, Sarim FM, Int. J. Biol. Macromol. , 147 , 439, 2019
Kamran U, Bhatti HN, Iqbal M, Jamil S, Zahid M, J. Mol. Struct. , 1179 , 532, 2019
Liu MY, Zhang XT, Li ZH, Qu LB, Han RP, Carbohydr. Polym. , 248 , 116792, 2020
Gu YF, Yang MM, Wang WL, Han RP, J. Chem. Eng. Data , 64 (6), 2849, 2019
Yuchi A, Ogiso A, Muranaka S, Niwa T, Anal. Chim. Acta , 494 , 81, 2003
He YH, Lin H, Dong YB, Wang L, Appl. Surf. Sci. , 426 , 995, 2017
Du WY, Li Y, Xu X, Shang YA, Gao BY, J. Colloid Interface Sci. , 9 , 2, 2018
Luo JM, Luo XB, Crittenden J, Qu JH, Bai YH, Peng Y, Li JH, Environ. Sci. Technol. , 18 , 1115, 2015
Mallet M, Barthelemy K, Ruby C, Renard A, Naille S, J. Colloid Interface Sci. , 407 , 95, 2013
Fang LP, Huang LZ, Holm PE, Yang XF, Hansen HCB, Wang D, J. Mater. Chem. A , 3 , 75055, 2015
Wu K, Li Y, Liu T, Huang QB, Yang SJ, Wang WD, Jin PK, Appl. Surf. Sci. , 478 , 539, 2019
Yan LG, Xu YY, Yu HQ, Xin XD, Wei Q, Du B, J. Hazard. Mater. , 179 (1-3), 244, 2010
Huang WW, Wang SB, Zhu ZH, Li L, Yao XD, Rudolph V, Haghseresht F, J. Hazard. Mater. , 158 (1), 35, 2008
Long F, Gong JL, Zeng GM, Chen L, Wang XY, Deng JH, Niu QY, Zhang HY, Zhang XR, Chem. Eng. J. , 171 (2), 448, 2011
Ren ZM, Shao LN, Zhang GS, Water Air Soil Pollut. , 223 , 4221, 2012
Zhao BL, Xiao W, Shang Y, Zhu HM, Han RP, Arab. J. Chem. , 10 , s359, 2017
Zhang XT, Ma CH, Wen K, Han R, Korean J. Chem. Eng. , 37 (5), 776, 2020
Chen BD, Wang J, Kong LJ, Mai XX, Zheng NC, Zhong QH, Liang JY, Chen DY, Colloids Surf. A: Physicochem. Eng. Asp. , 520 , 612, 2017
Rong Y, Han R, Korean J. Chem. Eng. , 36 (6), 942, 2019
Hu YY, Han RP, J. Chem. Eng. Data , 64 (2), 791, 2019
Yang YQ, Wen DW, Ding Q, Wang Y, Liu N, Zhao Y, Zhang X, Desalin. Water Treat. , 88 , 257, 2017
Zhang RD, Zhang JH, Zhang XN, Dou CC, Han RP, J. Taiwan Inst. Chem. Eng. , 45 , 2578, 2014
Chen ZH, Zhang JN, Fu JW, Wang MH, Wang XZ, Han RP, Xu Q, J. Hazard. Mater. , 273 , 263, 2014
Aryee AA, Mpatani FM, Zhang XT, Kani AN, Dovi AN, Dovi E, Han RP, Li ZH, Qu LB, J. Clean Prod. , 268 , 122191, 2020
Bhatti HN, Safa Y, Yakout SM, Shair OH, Iqbal M, Nazir A, Int. J. Biol. Macromol. , 150 , 861, 2020
Han MY, Zhang JH, Hu YY, Han RP, J. Chem. Eng. Data , 64 (8), 3641, 2019
Zhou T, Lu WZ, Liu LF, Zhu HM, Jiao YB, Zhang SS, Han RP, J. Mol. Liq. , 211 , 909, 2015
Zong EM, Wei D, Wan HQ, Zheng SR, Xu ZY, Zhu DQ, Chem. Eng. J. , 221 , 193, 2013
Lin JW, Wang XX, Zhan YH, J. Environ. Sci. , 76 , 167, 2019
Zhang XT, Zhang RZ, Chen SS, Wen K, Han RP, Desalin. Water Treat. , 170 , 187, 2019
Li JY, Ma J, Guo QH, Zhang SL, Han HY, Zhang SS, Han RP, Water Sci. Technol. , 81 , 824, 2020
Wu K, Li Y, Liu T, Huang QB, Yang SJ, Wang WD, Jin PK, Appl. Surf. Sci. , 478 , 539, 2019
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