Korean Journal of Chemical Engineering, Vol.35, No.7, 1532-1541, 2018
Immobilized titanium dioxide/powdered activated carbon system for the photocatalytic adsorptive removal of phenol
Titanium dioxide (TiO2) and powdered activated carbon (PAC) were fabricated via a layer by layer arrangement on a glass plate using a dip-coating technique for the photocatalytic-adsorptive removal of phenol. Thinner TiO2 layer coated on PAC sub-layer has larger surface area and better phenol removal than the thicker TiO2 layer. The system obeyed the Langmuir isotherm model, which exhibited a homogeneous and monolayer adsorption with a maximum capacity of 27.8mg g-1. The intra-particle diffusion was the rate-limiting step as the linear plot crossed the origin, while the adsorption was unfavorable at elevated temperature. Under light irradiation, the TiO2/PAC system removed phenol two-times more effectively than the TiO2 monolayer due to the synergistic effect of photocatalysis by TiO2 top layer and adsorption by PAC sub-layer. The COD removal of phenol was rapid for 10mg L-1 of concentration and under solar light irradiation. It was shown that the PAC sub-layer plays a significant role in the total removal of phenol by providing the adsorption sites and slowing down the recombination rate of charge carriers to improve the TiO2 photocatalytic oxidation performance.
[References]
Saravanan P, Pakshirajan K, Saha P, J. Hydro-environ. Res. , 3 , 45, 2009
Duma V, Popp KE, Kung MC, Zhou H, Nguyen S, Ohyama S, Kung HH, Marshall CL, Chem. Eng. J. , 99 (3), 227, 2004
Guo ZF, Ma RX, Li GJ, Chem. Eng. J. , 119 (1), 55, 2006
Fierascu I, Avramescu SM, Petreanu I, Marinoiu A, Soare A, Nica A, Fierascu RC, React. Kinet. Mech. Cat. , 122 , 155, 2017
Girods P, Dufour A, Fierro V, Rogaume Y, Rogaume C, Zoulalian A, Celzard A, J. Hazard. Mater. , 166 (1), 491, 2009
Mahadevan H, Dev VV, Krishnan KA, Abraham A, Ershana O, Environ. Technol. Innovation , 9 , 1, 2018
Baldrick P, Regul. Toxicol. Pharmacol. , 56 , 290, 2010
Saran S, Manjari G, Arunkumar P, Devipriya SP, Korean J. Chem. Eng. , 34 (11), 2984, 2017
Dong H, Zeng G, Tang L, Fan C, Zhang C, He X, He Y, Water Res. , 79 , 128, 2015
Farzadkia M, Shahamat YD, Nasseri S, Mahvi AH, Gholami M, Shahryari A, J. Eng. , 2014 , 10, 2014
Dubber D, Gray NF, J. Environ. Sci. Health Part A-Toxic/Hazard. Subst. Environ. Eng. , 45 , 1595, 2010
Rangkooy HA, Pour MN, Dehaghi BF, Korean J. Chem. Eng. , 34 (12), 3142, 2017
Kalantary RR, Shahamat YD, Farzadkia M, Esrafili A, Asgharnia H, Desalin. Water Treat. , 55 , 555, 2015
Omo-Okoro PN, Daso AP, Okonkwo JO, Environ. Technol. Innovation , 9 , 100, 2018
Sriwong C, Wongnawa S, Patarapaiboolchai O, J. Environ. Sci. , 24 , 464, 2012
Andriantsiferana C, Mohamed EF, Delmas H, Environ. Technol. , 35 , 355, 2014
Xing B, Shi C, Zhang C, Yi G, Chen L, Guo H, Huang G, Cao J, J. Nanomater , 2016 , 10, 2016
Martins AC, Cazetta AL, Pezoti O, Souza JRB, Zhang T, Pilau EJ, Asefa T, Almeida VC, Ceram. Int. , 43 , 4411, 2017
Ngoh YS, Nawi MA, Mater. Res. Bull. , 76 , 8, 2016
Jawad AH, Nawi MA, React. Kinet. Mech. Cat. , 106 , 49, 2012
Shi J, Zheng J, Wu P, Ji X, Catal. Commun. , 9 , 1846, 2008
Puma GL, Bono A, Krishnaiah D, Collin JG, J. Hazard. Mater. , 157 (2-3), 209, 2008
Andronic L, Duta A, Thin Solid Films , 515 (16), 6294, 2007
Lopez A, Acosta D, Martinez AI, Santiago J, Powder Technol. , 202 (1-3), 111, 2010
Stefanov B, Osterlund L, Coatings , 4 , 587, 2014
Zafar M, Yun JY, Kim DH, Korean J. Chem. Eng. , 35 , 567, 2017
Bahrudin NN, Nawi MA, React. Kinet. Mech. Cat. , 124 , 153, 2018
Nawi MA, Zain SM, Appl. Surf. Sci. , 258 (16), 6148, 2012
Marrakchi F, Khanday W, Asif M, Hameed B, Int. J. Biol. Macromol. , 93 , 1231, 2016
Xing B, Shi C, Zhang C, Yi G, Chen L, Guo H, Huang G, Cao J, J. Nanomater , 2016 , 3, 2016
Dada A, Olalekan A, Olatunya A, Dada O, IOSR J. Appl. Chem. , 3 , 38, 2012
Nethaji S, Sivasamy A, Mandal A, Int. J. Environ. Sci. Technol. , 10 , 231, 2013
Heraldy E, Hidayat Y, Firdaus M, IOP Conf. Series: Mater. Sci. Eng. , 107 , 012067, 2016
Ngoh YS, Nawi MA, Int. J. Environ. Sci. Technol. , 13 , 907, 2016
Nawi MA, Sabar S, Jawad AH, Sheilatina, Ngah WSW, Biochem. Eng. J. , 49 , 317, 2010
Ansari R, Mohammad-khah, Nazmi M, Current Chem. Lett. , 2 , 215, 2013
Jing LQ, Qu YC, Wang BQ, Li SD, Jiang BJ, Yang LB, Fu W, Fu HG, Sun JZ, Sol. Energy Mater. Sol. Cells , 90 (12), 1773, 2006
Sabar S, Nawi MA, Desalin. Water Treat. , 57 , 10312, 2016
Nawi MA, Sabar S, Sheilatina, J. Colloid Interface Sci. , 372 , 80, 2012
Ghosh T, Oh WC, Asian J. Chem. , 24 , 5419, 2012
Shahamat YD, Farzadkia M, Nasseri S, Mahvi AH, Gholami M, Esrafili A, J. Environ. Health Sci. Eng. , 12 , 50, 2014
Chen J, Zhang J, Xian Y, Ying X, Liu M, Jin L, Water Res. , 39 , 1340, 2005
Kang YW, Cho MJ, Hwang KY, Water Res. , 33 , 1247, 1999
Kolb M, Bahadir M, Teichgraber B, Water Res. , 122 , 645, 2017
Jin P, Chang R, Liu D, Zhao K, Zhang L, Ouyang Y, J. Environ. Chem. Eng. , 2 , 1040, 2014
Baransi K, Dubowski Y, Sabbah I, Water Res. , 46 , 789, 2012
[Cited By]
Bahrudin NN, Nawi MA, Korean Journal of Chemical Engineering , 36 (3), 478, 2019
Gao HS, Zong ZM, Yang Z, Teng DG, Sun XH, Yan L, Wei XY, Guo QJ, Zhao TS, Bai HC, Korean Journal of Chemical Engineering , 37 (5), 835, 2020
이전 논문 다음 논문
Result Search