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- In relation to this article, we declare that there is no conflict of interest.
- Publication history
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Received November 29, 2024
Accepted December 14, 2024
Available online June 25, 2025
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.
Latest issues
Designing Si Anode in Sulfi de-Based All-Solid-State Batteries: Insights from Established Strategies in Lithium-Ion Batteries
https://doi.org/10.1007/s11814-024-00364-2
Abstract
Silicon (Si) has attracted signifi cant interest as a promising anode material for all-solid-state batteries (ASSBs) due to its
exceptional potential to address safety concerns and enhance energy density. However, despite the diff erence in confi guration
between sulfi de-based ASSBs and lithium-ion batteries (LIBs), the degradation mechanism of Si anode in both systems
exhibit similarities, primarily attributed to the volume change of Si during (de)lithiation. Herein, beginning by fi guring out
the unique electrochemical behavior of Si anode in sulfi de-based ASSBs, which arises from the distinct solid–solid interface
dynamics, the recent comprehensive strategies are explored for the eff ective integration of Si anodes in sulfi de-based
ASSBs. By deepening our understanding of the failure mechanism of Si anode in sulfi de-based ASSBs and drawing from
well-established strategies developed for Si anodes in LIBs, we propose actionable insights for overcoming the limitation
of Si anode in sulfi de-based ASSBs.
