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In relation to this article, we declare that there is no conflict of interest.
Publication history
Received June 8, 2024
Accepted August 24, 2024
Available online January 25, 2025
articles This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.
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Thermal Analysis of the Gelation Process of Li-ion Battery Polymer Electrolyte by Electron Irradiation Using Multi-physics Simulation

Department of Nuclear Engineering , Kyung Hee University 1Department of Chemical Engineering , Hongik University
Korean Journal of Chemical Engineering, January 2025, 42(1), 165-177(13)
https://doi.org/10.1007/s11814-024-00271-6

Abstract

Rechargeable lithium-based batteries play a crucial role in the shift towards renewable energy, providing eco-friendly alternatives

to fossil fuels and improving sustainability. However, their liquid electrolytes present signifi cant safety risks, especially

in electric vehicles. To address this, the process of gelation through cross-linking has emerged as a promising solution, eff ectively

reducing the risk of combustion. Traditional gelation methods are time-consuming and costly, often taking up to an

hour. In contrast, electron beam irradiation provides a highly effi cient alternative, reducing the process to just seconds. This

lowers production costs and meets the demands of high-volume manufacturing. In this study, the multiphysical phenomena

in the coin cell were simulated using, which combines radiation transport modeling, phase change simulation of the gelation

process, and thermal analysis. Through this, the peak temperature of the electrolyte in the coin cell was predicted and the

time required for the temperature of the electrolyte to return to the ambient temperature was predicted.

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