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In relation to this article, we declare that there is no conflict of interest.
Publication history
Received June 16, 2024
Accepted June 24, 2024
articles This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.
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Ultrathin Glass-Based Perovskite Solar Cells Employing Bilayer Electron Transport Layer

Department of Chemical Engineering , Hanyang University
mjko@hanyang.ac.kr
Korean Journal of Chemical Engineering, December 2024, 41(14), 3791-3798(8)
https://doi.org/10.1007/s11814-024-00213-2

Abstract

In recent studies, fl exible perovskite solar cells (PSCs) have exhibited high power conversion effi ciency (PCE) coupled with

remarkable mechanical stability. However, the conventional polymer substrates used in fl exible PSCs possess high permeability

to moisture and oxygen, leading to the rapid degradation of perovskite materials. In this work, we address these

issues by employing ultrathin glass (UTG) substrates, which provide moisture impermeability while retaining fl exibility.

Additionally, we introduce a strategically designed SnO 2 /TiO 2 bilayer as the electron transport layer (ETL). Our results

reveal that PSCs incorporating the bilayer ETL achieve higher PCE than those with a monolayer ETL on conventional glass

and UTG substrates. Furthermore, moisture permeability tests demonstrate that PSCs based on UTG substrates sustain their

PCE over time, compared to their polymer-based counterparts. These results imply that UTG substrates, combined with a

SnO 2 /TiO 2 bilayer ETL, off er a promising solution for developing durable, high-performance, fl exible PSCs suitable for

long-term applications.

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