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Received November 3, 2016
Accepted April 18, 2017
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Anti-corrosive performance of epoxy coatings containing various nano-particles for splash zone applications
Center of Excellence for Research in Engineering Materials (CEREM), Advanced Manufacturing Institute (AMI), King Saud University, P. O. Box 800, Riyadh-11421, Saudi Arabia 1Chemical Engineering Department, King Saud University, P. O. Box 800, Riyadh-11421, Saudi Arabia 2Research Centre-College of Science, King Saud University, P. O. Box 2455, Riyadh-11451, Saudi Arabia
malamiitd@gmail.com
Korean Journal of Chemical Engineering, August 2017, 34(8), 2301-2310(10), 10.1007/s11814-017-0114-1
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Abstract
Various formulations of epoxy nano-composites coating were developed by incorporating the nanoparticles (NPs) of ZnO, ZrO2, and SiO2 (2 wt%) in commercially available epoxy resin as the matrix phase. Direct incorporation method was used for the addition of NPs in epoxy matrix. High-speed mechanical stirring and ultra-sonication were carried out to facilitate the dispersion of NPs in the presence of acetone used as a solvent. Coating of neat epoxy and NPs (ZnO, ZrO2, SiO2) doped coating was applied on mild steel substrate for corrosion analysis. The effect of the incorporation of various NPs on anti-corrosive properties of the epoxy/nano-composite coatings was investigated by electrochemical impedance spectroscopy technique. The experimental results showed an improvement in the anticorrosive properties for EZr coatings as compared with pristine and other nanocomposite coating samples.
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Ferreira ES, Giacomelli C, Giacomelli FC, Spinelli A, Mater. Chem. Phys., 853, 129 (2004)
Popovic MM, Grgur BN, Miskovic-Stankovic VB, Prog. Org. Coat., 52, 359 (2005)
Pennington BD, Grunlan JC, Urban MW, J. Coat. Technol., 71, 135 (1999)
Ates M, J. Adhes. Sci. Technol., 30(14), 1510 (2016)
Leidheiser H, Corrosion, 38, 374 (1982)
Walter GA, Corrosion Sci., 26, 27 (1986)
Van Westing EPM, Ferrari GM, De Wit JHW, Corrosion Sci., 34, 1511 (1993)
Hornstrom SE, Karlsson J, VanOoij WJ, Tang N, Klang H, J. Adhes. Sci. Technol., 10(9), 883 (1996)
Ji WG, Hu JM, Liu L, Zhang JQ, Cao CN, J. Adhes. Sci. Technol., 22(1), 77 (2008)
Rosero-Navarro NC, Pellice SA, Duran A, Aparicio M, Corrosion Sci., 20, 1283 (2008)
Huang TC, Su YA, Yeh TC, Huang HY, Wu CP, Huang KY, Chou YC, Yeh JM, Wei Y, Electrochim. Acta, 56(17), 6142 (2011)
Ma L, Chen F, Li Z, Gan M, Yan J, Wei S, Bai Y, Zeng J, Compos. Sci. Technol., 58, 54 (2014)
Shi H, Liu F, Yang L, Han E, Prog. Org. Coat., 62, 359 (2008)
Mahulikar PP, Jadhav RS, Hundiwale DG, Iran. Polym. J., 20, 367 (2011)
Balaskas AC, Kartsonakis IA, Tziveleka LA, Kordas G, Prog. Org. Coat., 74, 418 (2012)
Kouloumbi N, Tsangaris GM, Vourvahi C, Molnar F, J. Coat. Technol., 69, 53 (1997)
Veleva L, Chin J, Del Amo B, Prog. Org. Coat., 36, 211 (1999)
Rashvand M, Ranjbar Z, Rastegar S, J. Electrochem. Soc., 159(3), C129 (2012)
Dhoke SK, Khanna A, Sinha TJM, Prog. Org. Coat., 64, 371 (2009)
Ehsani A, Mahjani MG, Nasseri M, Jafarian M, Anti-Corros. Method. M., 61, 146 (2014)
Dhoke SK, Sinha TJM, Khanna A, J. Coat. Technol., 6, 353 (2009)
Gusmano G, Montesperelli G, Rapone M, Padeletti G, Cusma A, Kaciulis S, Mezzi A, Surf. Coat. Technol., 201, 5822 (2007)
Alexandre M, Dubois P, Mater. Sci. Eng. R-Rep., 28, 1 (2000)
Chaiko DJ, Leyva AA, Chem. Mater., 17, 19 (2005)
Sabzi M, Mirabedini S, Zohuriaan-Mehr J, Atai M, Prog. Org. Coat., 65, 222 (2009)
Gerosa M, Sacco A, Scalia A, Bella F, Chiodoni A, Quaglio M, Tresso E, Bianco S, IEEE J. Photovolt., 6, 498 (2016)
Bella F, Sacco A, Massaglia G, Chiodoni A, Pirri CF, Quaglio M, Nanoscale., 7, 12010 (2015)
Bella F, Leftheriotis G, Griffini G, Syrrokostas G, Turri S, Gratzel M, Gerbaldi C, Adv. Funct. Mater., 26(7), 1127 (2016)
Im P, Choi YJ, Yoon WJ, Kang DG, Park M, Kim DY, Lee CR, Yang S, Lee JH, Jeong K, Sci. Rep., 6, 36472 (2016)
Pintossi D, Iannaccone G, Colombo A, Bella F, Valimaki M, Vaisanen KL, Hast J, Levi M, Gerbaldi C, Dragonetti C, Turri S, Griffni G, Adv. Electron. Mater., 2, 160028 (2016)
Nakagawa M, Nakaya A, Hoshikawa Y, Ito S, Hiroshiba N, Kyotani T, ACS Appl. Mater. Interfaces., 8, 30628 (2016)
Ramezanzadeh B, Attar MM, Farzam M, Prog. Org. Coat., 72, 410 (2011)
Ramezanzadeh B, Attar MM, Prog. Org. Coat., 71, 242 (2011)
Huang ZM, Mater. Sci. Technol., 16, 81 (2000)
Ramezanzadeh B, Attar MM, Farzam M, J. Therm. Anal. Calorim., 103, 731 (2011)
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Ramezanzadeh B, Attar MM, Farzam M, Prog. Org. Coat., 72, 410 (2011)
Khan R, Azhar MR, Anis A, Alam MA, Boumaza M, Al-Zahrani SM, J. Coat. Technol., 13, 159 (2016)
Wu J, Xie J, Ling L, Ma G, Wang B, J. Coat. Technol., 10, 849 (2013)
Choi J, Kim SG, Laine RM, Macromolecules, 37(1), 99 (2004)
Gilman JW, Jackson CL, Morgan AB, Harris R, Manias E, Giannelis EP, Wuthenow M, Hilton D, Phillips SH, Chem. Mater., 12, 1866 (2000)
Peng Z, Kong LX, Li SD, J. Appl. Polym. Sci., 96(4), 1436 (2005)
Hsu SC, Whang WT, Hung CH, Chiang PC, Hsiao YN, Macromol. Chem. Phys., 206, 291 (2005)
Mirabedini SM, Thompson GE, Moradian S, Scantlebury JD, Prog. Org. Coat., 46, 112 (2003)
Niknahad M, Moradian S, Mirabedini SM, Corrosion Sci., 52, 1948 (2010)
Walter GW, Corrosion Sci., 26, 681 (1986)
Mirabedini SM, Behzadnasab M, Kabiri K, Compos. Pt. A-Appl. Sci. Manuf., 43, 2095 (2012)
Sanchez MS, Mateo JM, Colomer FJR, Ribelles JLG, Eur. Polym. J., 42, 1378 (2006)
Chattopadhyay DK, Muehlberg AJ, Webster DC, Prog. Org. Coat., 63, 405 (2008)
Kim SW, Korean J. Chem. Eng., 25(5), 1195 (2008)
Kim SW, Korean J. Chem. Eng., 28(1), 298 (2011)
