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Issue
Korean Journal of Chemical Engineering,
Vol.38, No.11, 2247-2255, 2021
Fabrication and modification of cellulose aerogels from Vietnamese water hyacinth for oil adsorption application
Phat LN, Thang TQ, Nguyen HC, Duyen DTM, Tien DX, Khoa BDD, Khang PT, Giang NTH, Nam HM, Phong MT, Hieu NH
Recycling biomass to cellulose aerogel (Cell-A) provides a promising approach to develop adsorbent materials for spilled-oil recovery. In this work, Cell-A was fabricated from Vietnamese water hyacinth via crosslinking methods using PVA as a crosslinker and freeze-drying process. Various cellulose to PVA ratios were investigated to obtain the optimal synthesis condition. The Cell-A was additionally modified by dip-coating in poly(dimethylsiloxane) (PDMS) and pyrolyzing to form PDMS-coated cellulose aerogels (Cell-AP) and carbon aerogels (CA), respectively. Results of the oil adsorption tests show that pyrolysis produced aerogels with greater adsorption capacity with an optimal mass ratio of 15 : 1 cellulose to PVA. Furthermore, the pseudo-second-order model was found to be more accurate than the pseudo-first-order model for the study of oil absorption kinetics. As a result, the modified cellulose aerogel is promising for replacing earth-unfriendly polymer-based oil sorbents due to their high oil absorption capacity.
Keywords: Oil-spill Cleaning; Oil Adsorbent; Aerogel Materials; Biomass Recycling
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